As the standards movement continues into its third decade, there remains a need for alignment methodologies that can be broadly applied to study instruction and policy. This article reports on a series of development efforts meant to revise the Surveys of Enacted Curriculum (SEC) surveys and methods to study the implementation of new college- and career-readiness standards. The work included a meeting of content experts, a series of cognitive interviews, two validation studies, and a small pilot. We discuss both the results of the specific studies and the implications of the work for other potential users of the SEC or SEC-like tools. [For the corresponding Grantee Submission, see ED604916.]