The use of "Origami" is presented as an accessible and transferable modeling system through which to convey the intricacies of molecular shape and highlight structure-function relationships. The implementation of origami has been found to be a versatile alternative to conventional ball-and-stick models, possessing the key advantages of being both inexpensive and readily accessible. The challenge, tangible nature, sense of achievement and hence trophy-like status of the models were found to combine and serve as a potentially invaluable outreach resource in terms of transfer to the home environment, with most (greater than 70%) participants) wishing to show them to friends and family. A range of models were constructed and their implementation as lecture aids in both secondary and tertiary curricula has been assessed. (Contains 6 figures.)