Max Weber is seen by mainstream social scientists as a sociologist, social theorist, and theorist of bureaucracy. In this reassessment of Weber's social science and its methodology, it is suggested that Weber can also be seen as a compelling early 20th-century critic of science and technology. The theme of technology, and Webers ambivalence about it, is approached through a discussion of his notion of disenchantment. In the modern, disenchanted world, social scientists are compelled to choose the values that guide research, but research is constrained by the technocratic requirements of large, bureaucratic institutions that sponsor and fund it. The article asks whether Weber's notion of individual values is still applicable in the context of social science in the early 21st century. In a line of thought that can be traced to Postman and Ellul, it is asked whether the choices social scientists make can puncture the dense web of bureaucratic-technological rationality of which Weber was critical.